Overview

In the angle-resolved cathodoluminescence (ARCL) mode, the direction in which a photon is emitted is determined. An objective lens or, more commonly, a collection mirror projects an image of the emitted light onto a pixelated detector, e.g., a camera. When an appropriate optical system is used, each pixel in the captured image corresponds to a unique emission direction from the specimen. Typically, the raw image is transformed into polar coordinates for display and interpretation.

The result of an angle-resolved measurement contains no wavelength or polarization information unless additional filtering of dispersion is used (e.g., wavelength- and angle-resolved mode).

Angle-filtered information may be captured by using an iris or a pinhole to select a certain (range of) angle(s). However, the low resolution and highly serial nature of this particular acquisition mode have limited its usefulness.

Sometimes referred to as Fourier imaging or momentum spectroscopy.


Schematic ray diagrams demonstrating the experimental setup for intensity (left) and angle-resolved (right) measurements. A specialized optical system is required for angle-resolved measurements with the transfer optics and detector changed such that a 2D image is projected and sensed by a pixelated detector.

Data collection

Emission pattern or angle-resolved emission pattern: The emission pattern is a plot of the direction in which photons are emitted from a specimen, typically presented in polar coordinates where the emission direction is described by the azimuthal and zenith angles. A single emission pattern may be captured from a point or region of the sample exposed to the electron beam of the electron microscope.

Emission pattern image or angle-resolved spectrum image: The electron beam is scanned across the specimen surface, and an emission pattern is recorded at each location, creating a hyperspectral (4D) data construct.

Uses

To understand the emission pattern of light-emitting devices and how light and matter interact far below the optical diffraction limit. See the full experiment brief. 


A polarization-filtered angle-resolved composite result from Au-Pd nanostar.